Beta-decay stable isobars

Beta-decay stable isobars are the set of nuclides which cannot undergo beta decay, that is, the transformation of a neutron to a proton or a proton to a neutron within the nucleus. A subset of these nuclides are also stable with regards to double beta decay or theoretically higher simultaneous beta decay, as they have the lowest energy of all nuclides with the same mass number.

This set of nuclides is also known as the line of beta stability, a term already in common use in 1965.[1][2] This line lies along the bottom of the nuclear valley of stability.

Introduction

The line of beta stability can be defined mathematically by finding the nuclide with the greatest binding energy for a given mass number, by a model such as the classical semi-empirical mass formula developed by C. F. Weizsäcker. These nuclides are local maxima in terms of binding energy for a given mass number.

β decay stable / even N
#βDS:OneTwoThree
2-3417
36-5857
60-7252
74-1162191
118-1542116
156-192514
194-21063
212-260619
Total48757

All odd mass numbers have only one beta decay stable nuclide.

Among even mass number, seven (96, 124, 130, 136, 148, 150, 154) have three beta-stable nuclides. None have more than three, all others have either one or two.

All primordial nuclides are beta decay stable, with the exception of 40K, 50V, 87Rb, 113Cd, 115In, 138La, 176Lu, and 187Re. In addition, 123Te and 180mTa have not been observed to decay, but are believed to undergo beta decay with an extremely long half-life (over 1015 years). All elements up to and including nobelium, except technetium and promethium, are known to have at least one beta-stable isotope.

List of known beta-decay stable isobars

Theoretically predicted or experimentally observed double beta-decay (if not dominated by alpha decay or spontaneous fission) is shown by arrows, i.e. arrows point towards the lightest-mass isobar. There are currently known to be 358 beta-decay stable nuclides.[3]

Even NOdd N
Even ZEven AOdd A
Odd ZOdd AEven A
All beta-decay stable isobars with A ≤ 260 sorted by mass number
Odd AEven AOdd AEven AOdd AEven AOdd AEven A
1H 2H 3He 4He 5He (n) 6Li 7Li 8Be (α)
9Be 10B 11B 12C 13C 14N 15N 16O
17O 18O 19F 20Ne 21Ne 22Ne 23Na 24Mg
25Mg 26Mg 27Al 28Si 29Si 30Si 31P 32S
33S 34S 35Cl 36S ← 36Ar 37Cl 38Ar 39K 40Ar ← 40Ca
41K 42Ca 43Ca 44Ca 45Sc 46Ca → 46Ti 47Ti 48Ca → 48Ti
49Ti 50Ti ← 50Cr 51V 52Cr 53Cr 54Cr ← 54Fe 55Mn 56Fe
57Fe 58Fe ← 58Ni 59Co 60Ni 61Ni 62Ni 63Cu 64Ni ← 64Zn
65Cu 66Zn 67Zn 68Zn 69Ga 70Zn → 70Ge 71Ga 72Ge
73Ge 74Ge ← 74Se 75As 76Ge → 76Se 77Se 78Se ← 78Kr 79Br 80Se → 80Kr
81Br 82Se → 82Kr 83Kr 84Kr ← 84Sr 85Rb 86Kr → 86Sr 87Sr 88Sr
89Y 90Zr 91Zr 92Zr ← 92Mo 93Nb 94Zr → 94Mo 95Mo 96Zr → 96Mo ← 96Ru
97Mo 98Mo → 98Ru 99Ru 100Mo → 100Ru 101Ru 102Ru ← 102Pd 103Rh 104Ru → 104Pd
105Pd 106Pd ← 106Cd 107Ag 108Pd ← 108Cd 109Ag 110Pd → 110Cd 111Cd 112Cd ← 112Sn
113In 114Cd → 114Sn 115Sn 116Cd → 116Sn 117Sn 118Sn 119Sn 120Sn ← 120Te
121Sb 122Sn → 122Te 123Sb 124Sn → 124Te ← 124Xe 125Te 126Te ← 126Xe 127I 128Te → 128Xe
129Xe 130Te → 130Xe ← 130Ba 131Xe 132Xe ← 132Ba 133Cs 134Xe → 134Ba 135Ba 136Xe → 136Ba ← 136Ce
137Ba 138Ba ← 138Ce 139La 140Ce 141Pr 142Ce → 142Nd 143Nd 144Nd (α) ← 144Sm
145Nd 146Nd → 146Sm (α) 147Sm (α) 148Nd → 148Sm (α) ← 148Gd (α) 149Sm 150Nd → 150Sm ← 150Gd (α) 151Eu (α) 152Sm ← 152Gd
153Eu 154Sm → 154Gd ← 154Dy (α) 155Gd 156Gd ← 156Dy 157Gd 158Gd ← 158Dy 159Tb 160Gd → 160Dy
161Dy 162Dy ← 162Er 163Dy 164Dy ← 164Er 165Ho 166Er 167Er 168Er ← 168Yb
169Tm 170Er → 170Yb 171Yb 172Yb 173Yb 174Yb ← 174Hf 175Lu 176Yb → 176Hf
177Hf 178Hf 179Hf 180Hf ← 180W (α) 181Ta 182W 183W 184W ← 184Os (α)
185Re 186W → 186Os (α) 187Os 188Os 189Os 190Os ← 190Pt (α) 191Ir 192Os → 192Pt
193Ir 194Pt 195Pt 196Pt ← 196Hg 197Au 198Pt → 198Hg 199Hg 200Hg
201Hg 202Hg 203Tl 204Hg → 204Pb 205Tl 206Pb 207Pb 208Pb
209Bi (α) 210Po (α) 211Po (α) 212Po (α) ← 212Rn (α) 213Po (α) 214Po (α) ← 214Rn (α) 215At (α) 216Po (α) → 216Rn (α)
217Rn (α) 218Rn (α) ← 218Ra (α) 219Fr (α) 220Rn (α) → 220Ra (α) 221Ra (α) 222Ra (α) 223Ra (α) 224Ra (α) ← 224Th (α)
225Ac (α) 226Ra (α) → 226Th (α) 227Th (α) 228Th (α) 229Th (α) 230Th (α) ← 230U (α) 231Pa (α) 232Th (α) → 232U (α)
233U (α) 234U (α) 235U (α) 236U (α) ← 236Pu (α) 237Np (α) 238U (α) → 238Pu (α) 239Pu (α) 240Pu (α)
241Am (α) 242Pu (α) ← 242Cm (α) 243Am (α) 244Pu (α) → 244Cm (α) 245Cm (α) 246Cm (α) 247Bk (α) 248Cm (α) → 248Cf (α)
249Cf (α) 250Cf (α) 251Cf (α) 252Cf (α) ← 252Fm (α) 253Es (α) 254Cf (SF) → 254Fm (α) 255Fm (α) 256Fm (SF)
257Fm (α) 258Fm (SF) ← 258No (SF) 259Md (SF) 260Fm (SF) → 260No (SF)
Known beta-decay stable isobars with A > 260 sorted by mass number
261No (α) 262No (SF) 263Lr (α) 264No (SF) → 264Rf (SF) 265Lr (SF) 266No (SF) → 266Rf (SF) 267Rf (SF) 268Rf (SF) 269Db (α, SF) 270Rf (SF)

All beta-decay stable nuclides with A ≥ 209 were observed to decay by alpha decay except some where spontaneous fission dominates.

261No, 263Lr, 264No, 264Rf, 265Lr, 266No, and 269Db have not yet been synthesized; the synthesis of 260Fm, 262No, 266Rf, 268Rf, and 270Rf is unconfirmed.

Further predicted beta-decay stable isobars are 272Sg, 275Bh, 278Hs, 281Mt, 284Ds, 287Rg, 290Cn, 293Nh, 296Fl, 299Mc, 302Lv, and 305Ts.[4]

Beta decay toward minimum mass

Beta decay generally causes isotopes to decay toward the isobar with the lowest mass (highest binding energy) with the same mass number, those not in italics in the table above. Thus, those with lower atomic number and higher neutron number than the minimum-mass isobar undergo beta-minus decay, while those with higher atomic number and lower neutron number undergo beta-plus decay or electron capture. However, there are four nuclides that are exceptions, in that the majority of their decays are in the opposite direction:

Chlorine-3635.96830698Potassium-4039.96399848Silver-108107.905956Promethium-146145.914696
2% to Sulfur-3635.9670807611.2% to Argon-4039.96238312253% to Palladium-108107.90389237% to Samarium-146145.913041
98% to Argon-3635.96754510689% to Calcium-4039.9625909897% to Cadmium-108107.90418463% to Neodymium-146145.9131169

References

  1. Proc. Int. Symposium on Why and How should we investigate Nuclides Far Off the Stability Line", Lysekil, Sweden, August 1966, eds. W. Forsling, C.J. Herrlander and H. Ryde, Stockholm, Almqvist & Wiksell, 1967
  2. Annual Review of Nuclear and Particle Science Vol. 29: 69-119 (Volume publication date December 1979) P G Hansen, "Nuclei Far Away from the Line of Beta Stability: Studies by On-Line Mass Separation" doi:10.1146/annurev.ns.29.120179.000441
  3. Interactive Chart of Nuclides (Brookhaven National Laboratory)
  4. https://arxiv.org/pdf/nucl-th/0512023v1.pdf
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